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            Abstract Sulfuryl fluoride (SO2F2) is a synthetic pesticide and a potent greenhouse gas that is accumulating in the global atmosphere. Rising emissions are a concern since SO2F2has a relatively long atmospheric lifetime and a high global warming potential. The U.S. is thought to contribute substantially to global SO2F2emissions, but there is a paucity of information on how emissions of SO2F2are distributed across the U.S., and there is currently no inventory of SO2F2emissions for the U.S. or individual states. Here we provide an atmospheric measurement-based estimate of U.S. SO2F2emissions using high-precision SO2F2measurements from the NOAA Global Greenhouse Gas Reference Network (GGGRN) and a geostatistical inverse model. We find that California has the largest SO2F2emissions among all U.S. states, with the highest emissions from southern coastal California (Los Angeles, Orange, and San Diego counties). Outside of California, only very small and infrequent SO2F2emissions are detected by our analysis of GGGRN data. We find that California emits 60-85% of U.S. SO2F2emissions, at a rate of 0.26 ( ± 0.10) Gg yr−1. We estimate that emissions of SO2F2from California are equal to 5.5–12% of global SO2F2emissions.more » « less
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            Abstract Despite the key role of the Arctic in the global Earth system, year-round in-situ atmospheric composition observations within the Arctic are sparse and mostly rely on measurements at ground-based coastal stations. Measurements of a suite of in-situ trace gases were performed in the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition. These observations give a comprehensive picture of year-round near-surface atmospheric abundances of key greenhouse and trace gases, i.e., carbon dioxide, methane, nitrous oxide, ozone, carbon monoxide, dimethylsulfide, sulfur dioxide, elemental mercury, and selected volatile organic compounds (VOCs). Redundancy in certain measurements supported continuity and permitted cross-evaluation and validation of the data. This paper gives an overview of the trace gas measurements conducted during MOSAiC and highlights the high quality of the monitoring activities. In addition, in the case of redundant measurements, merged datasets are provided and recommended for further use by the scientific community.more » « less
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            Noetzli, J., Christiansen, H.H, Guglielmin, M., Hrbáček, F., Hu, G., Isaksen, K., Magnin, F., Pogliotti, P., Smith, S. L., Zhao, L. and Streletskiy, D. A. 2024. Permafrost temperature and active layer thickness. In: State of the Climate in 2023. Bulletin of the American Meteorological Society, 105 (8), S43–S44, https://doi.org/10.1175/BAMS-D-24-0116.1more » « less
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